Visualizing Poiseuille flow of hydrodynamic electrons

We imaged hydrodynamic electron flow for the first time, observing how electrons can be made to flow through a graphene nanodevice like water through a pipe, with a higher current density at the center than near the walls.

Go to the profile of Joseph Sulpizio
Dec 04, 2019
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Hydrodynamics is an omnipresent phenomenon in the physical world, dictating the behavior of systems with many inter-particle collisions, such as the flow of classical fluids like water. The possibility of hydrodynamic flow of electrons, fundamental quantum particles, is especially exciting, as such new behavior would be in stark contrast to the long observed property that electrons flow through a material like a gas, either diffusively or ballistically.  From a more practical perspective, one can also imagine engineering new kinds of devices to exploit the nonlocal, viscous effects predicted to arise for hydrodynamic electrons, which might be advantageous for producing low-power, energy-efficient electronics.

The field of electron hydrodynamics dates back at least to the 1960s, when Radii Gurzhi considered theoretically how electrons might flow through a conductor that is free from impurities [1]. Indeed, in order to reach the hydrodynamic regime for electrons, a host material of extreme purity is required so that electrons will scatter off each other at a much higher rate than they scatter from disorder. Advances in the 80s in the creation of high-mobility two-dimensional electron gases (like those made from molecular beam epitaxy of semiconducting heterostructures), enabled Gurzhi’s predictions to be tested experimentally, and in a landmark paper in 1995 by de Jong and Molenkamp [2], signatures of electron hydrodynamics were finally observed in transport measurements of GaAs-based semiconducting wires.

Subsequently, the field largely stagnated for the next twenty years or so, only to be resurrected by the advent of high mobility van der Waals heterostructures such as graphene sandwiched between hexagonal boron nitride, which can be made exceptionally free from disorder. These materials inspired a new generation of researchers to consider the prospect of electron hydrodynamics, resulting in a flurry of activity, both experimental and theoretical. Still, while many new elements of electron hydrodynamics were being uncovered, the vast majority of the experimental work consisted of transport measurements that probe the devices at fixed spatial positions. Hydrodynamics, however, is a fundamentally spatial phenomenon, conjuring pictures of swirling fluids and raging waves (illustrated in figure 1). It was this challenge of actually visualizing the spatial aspects of electron hydrodynamics that initially drew us into the field.

Figure 1. Artist's conception of electron hydrodynamics, illustrated as a river of electrons flowing in graphene. The viscosity generated by the repulsion between electrons (red balls) causes them to flow with a parabolic current density, depicted by the white foam wavefront.

Just as the field of electron hydrodynamics was being revitalized, we were developing a new technique at the Weizmann Institute of Science for imaging electron flow in devices. Using a carbon nanotube single electron transistor as an ultrasensitive detector, we learned how to map the electrostatic potential of the flowing electrons inside a device to microvolt sensitivity [3], which is at least 1000 times more sensitive than other techniques such as Kelvin probe microscopy. Moreover, because our technique is capable of imaging electrons buried under insulating surfaces, across a broad temperature range (cryogenic to 300K), and in nonzero magnetic field, it seemed ideally suited for imaging electron hydrodynamics phenomena in van der Waals structures. We thus initiated a collaboration with the group of Andre Geim in Manchester to combine their state-of-the-art graphene devices with our unique imaging technique at Weizmann. The Manchester group were ideal partners, as they had already established the existence of electron hydrodynamics in graphene through transport measurements of the non-local resistance, and had built a solid theoretical understanding of this phenomenon.

We initially focused our efforts on imaging voltage whirlpools in graphene that were predicted to arise for hydrodynamic electrons, but we soon realized that ballistic effects could easily mimic the hydrodynamic flow we were aiming to study. To understand why this is the case, it helps to first discuss in more detail how the hydrodynamic regime can be accessed experimentally. Electrons in most materials are well-described by Fermi liquid theory, which explains that due to the Pauli exclusion principle, electrons at very low temperature behave essentially as if they are non-interacting, despite being negatively charged. If the electrons are heated, the phase space available for electron-electron scattering increases, and so heating can essentially “turn on” the repulsive interactions. However, electron flow in a typical material is actually dominated by disorder, and consequently electrons will scatter more rapidly from defects and impurities than from each other. This results in most materials obeying Ohm’s law. If a material is instead sufficiently clean, at low temperature electrons can largely flow without encountering any obstacles, only scattering at the device walls/edges. This is the ballistic transport regime, which can be achieved experimentally in materials like high-mobility graphene. If such a ballistic device is heated, then the hydrodynamic regime can be reached in which the rate of electron-electron scattering is much higher than the rate of scattering from impurities or from the device boundaries. Heating too much will introduce phonon scattering, reverting the system to the Ohmic regime.

Therefore, in order to confidently observe the hydrodynamic regime in experiment, we must be able to distinguish it from the ballistic regime from which it emerges. Ballistic electron flow, however, can easily produce complex spatial voltage patterns due to electrons bouncing off the device walls, and can even generate whirlpool-like features that are in fact much stronger than their hydrodynamic counterparts. This realization led us to augment our goal and instead aim for imaging the most fundamental spatial manifestation of hydrodynamic flow, the ‘Poiseuille’ flow profile.

Due to viscosity, when water flows through a pipe it flows faster at the center and slower at the walls, resulting in a parabolic velocity profile known as Poiseuille flow. Similarly, hydrodynamic electrons should also flow with higher current density near the center of a channel than at the walls. Observing this in experiment isn’t as straightforward as just imaging the current density, though, as we uncovered through simulation of electron flow through channels with the help of our theory colleagues. In contrast to the naïve expectation that the current density should be uniform in a ballistic channel, for the longest mean free paths at low temperature reached in experiment, the current density is actually not flat but is also parabolic. Reaching a flat current density requires an unphysically long mean free path, meaning that the current density itself does not sharply distinguish between ballistic and hydrodynamic flow.

It turns out that a much more discriminating metric is the spatial profile of the Hall electric field generated when a weak magnetic field is applied perpendicular to the direction of current flow. While this sounds fairly abstract, it’s simply the spatial derivative of the Hall voltage along the transverse direction, which is easily measured by our technique. In the ohmic regime, the Hall field is linearly proportional to the current density at the same spatial point (i.e. the classical Hall effect), and so the Hall field is essentially a measure of the local current density. This is also the case in the strongly hydrodynamic regime, where both the Hall field profile and the current density are predicted to be parabolic and locally proportional to each other. However, in the ballistic regime, while the current density profile can also be parabolic, the Hall field profile is flat.

For the experiments described in the paper [4], we flowed a current through our graphene channels under the application of a very weak magnetic field (so as to create a measureable Hall signal without influencing the flow) and imaged the resulting Hall field profiles. An optical image of a representative channel device and a sketch of the scanning measurement is shown in figure 2a,b. At low temperature (T=7.5K), we observe a flat Hall field profile consistent with ballistic transport (figure 2c). At elevated temperature (T=75K), we observe a strongly parabolic profile, indicating the transition to hydrodynamic flow (figure 2d). Moreover, because in the hydrodynamic regime the Hall field is equivalent to the current density, this measurement is actually the first image of Poiseuille flow of electrons. In the paper, we further explore the full temperature and carrier density dependence of the Hall field curvature, demonstrating how hydrodynamic electron flow evolves from ballistic flow.

Figure 2. Experimental imaging of Poiseuille electron flow. a, Optical image of graphene channel device. b, Schematic diagram of imaging experiment, with carbon nanotube single electron transistor scanning across graphene channel device. c, Experimental image of the Hall field at temperature T=7.5K taken over the region enclosed by the rectangle in a. The Hall field is flat across the bulk of the channel, indicating ballistic electron flow. d, Experimental image of the Hall field at temperature T=75K. At this elevated temperature, the Hall field is strongly parabolic due to electron-electron interactions (electron-electron scattering length lee ≈ 750nm). Because of the equivalence of the Hall field and the current density in the hydrodynamic regime, this image corresponds to a spatial map of the current density exhibiting Poiseuille electron flow (right z-axis is current density). Figure adapted from [4].

The revived field of electron hydrodynamics is still in its infancy, and the grounds for discovery remain fertile. In this work we imaged just one fundamental property of hydrodynamic electron flow, but using the richness of conventional hydrodynamics as a guide, there’s a vast array of electron hydrodynamics phenomena waiting to be revealed. For example, with carefully considered device design, it should soon be feasible to image hydrodynamic voltage whirlpools, and with future advancements in materials and device fabrication, it may even be possible to visualize turbulent electron flow as well. It's also interesting to consider how electron hydrodynamics may help us exceed conventional device performance limits (e.g. superballistic flow), as well as what role quantum mechanics may play in strongly interacting, hydrodynamic systems. Beyond hydrodynamics, our technique [3] holds a lot of promise for visualizing other interesting aspects of electron flow in nanostructures which previously could only be studied via transport.

For a different take on the work, check out the Nature News & Views feature here: Electrons in graphene go with the flow.

References

[1] Gurzhi, R. N. Minimum of resistance in impurity free conductors. Sov. Phys. JETP 17, 521 (1963).

[2] de Jong, M.J.M. & Molenkamp, L.W. Hydrodynamic electron flow in high-mobility wires. Phys. Rev. B 51, 13389-13402 (1995).

[3] Ella, L., Rozen, A., Birkbeck, J., Ben-Shalom, M., Perello, D., Zultak, J., Taniguchi, T., Watanabe, K., Geim, A.K., Ilani, S., & Sulpizio, J.A. Simultaneous imaging of voltage and current density of flowing electrons in two dimensions. Nature Nanotechnology 14, 480-487 (2019).

[4] Sulpizio, J.A., Ella, L., Rozen, A., Birkbeck, J., Perello, D.J., Dutta, D., Ben-Shalom, M., Taniguchi, T., Watanabe, K., Holder, T., Queiroz, R., Principi, A., Stern, A., Scaffidi, T., Geim, A.K., & Ilani, S. Visualizing Poiseuille flow of hydrodynamic electrons. Nature 576, 75-79 (2019).


Go to the profile of Joseph Sulpizio

Joseph Sulpizio

Research Scientist, Weizmann Institute of Science

PhD in physics from Stanford University, now in the department of Condensed Matter Physics at the Weizmann Institute of Science, researching new ways to image electrons in nanoscale devices and quantum materials.

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